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Modern Aspects of Diffusion-Controlled Reactions - Cooperative Phenomena in Bimolecular Processes (Cód: 3027556)

V. Kuzovkov; E. Kotomin

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Modern Aspects of Diffusion-Controlled Reactions - Cooperative Phenomena in Bimolecular Processes

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Descrição

This monograph deals with the effects of reactant spatial correlations arising in the course of basic bimolecular reactions describing defect recombination, energy transfer and exciton annihilation in condensed matter. These effects lead to the kinetics consideredabnormal from the standard chemical kinetics point of view. Numerous bimolecular reaction regimes and conditions are analysed in detail. Special attention is paid to the development and numerous applications of a novel, many-point density (MPD) formalism, which is based on Kirkwood'apos;s superposition approximation used for decoupling three-particle correlation functions.The book demonstrates that incorporation of the reaction-induced spatial correlations of similar reactants (e.g., vacancy-vacancy) leads to the development of an essentially non-Poisson spectrum of reactant density fluctuations. This can completely change the kinetics at longer times since it no longer obeys the law of mass action. The language of the correlation lengths and critical exponents similar to physics of critical phenomena is used instead. A relation between MPD theory and synergistics is discussed. The validity of the theorem giving a critical complexity for the two-step reactions exhibiting self-organization phenomena is questioned. Theoretical results are illustrated by numerous experimental data.

Características

Peso 0.00 Kg
Produto sob encomenda Sim
Marca ELSEVIER S&T
Idioma 337
Acabamento e-book
Territorialidade Internacional
Gratuito Não
Proteção Drm Sim
Tamanho do Arquivo 24647
Início da Venda 24/10/1996
Código do Formato Pdf
Cód. Barras 9780080536675
Ano da edição 101996
Ano da Publicação 1996
AutorV. Kuzovkov; E. Kotomin